Search results for "spin dynamics"
showing 10 items of 13 documents
Interaction-induced spin polarization in quantum dots.
2010
The electronic states of lateral many electron quantum dots in high magnetic fields are analyzed in terms of energy and spin. In a regime with two Landau levels in the dot, several Coulomb blockade peaks are measured. A zig-zag pattern is found as it is known from the Fock-Darwin spectrum. However, only data from Landau level 0 show the typical spin-induced bimodality, whereas features from Landau level 1 cannot be explained with the Fock-Darwin picture. Instead, by including the interaction effects within spin-density-functional theory a good agreement between experiment and theory is obtained. The absence of bimodality on Landau level 1 is found to be due to strong spin polarization.
Quasi-Lie Brackets and the Breaking of Time-Translation Symmetry for Quantum Systems Embedded in Classical Baths
2018
Many open quantum systems encountered in both natural and synthetic situations are embedded in classical-like baths. Often, the bath degrees of freedom may be represented in terms of canonically conjugate coordinates, but in some cases they may require a non-canonical or non-Hamiltonian representation. Herein, we review an approach to the dynamics and statistical mechanics of quantum subsystems embedded in either non-canonical or non-Hamiltonian classical-like baths which is based on operator-valued quasi-probability functions. These functions typically evolve through the action of quasi-Lie brackets and their associated Quantum-Classical Liouville Equations, or through quasi-Lie brackets a…
Lattice-Site-Specific Spin Dynamics in Double PerovskiteSr2CoOsO6
2014
Magnetic properties and spin dynamics have been studied for the structurally ordered double perovskite Sr2CoOsO6. Neutron diffraction, muon-spin relaxation, and ac-susceptibility measurements reveal two antiferromagnetic (AFM) phases on cooling from room temperature down to 2 K. In the first AFM phase, with transition temperature TN1=108 K, cobalt (3d7, S=3/2) and osmium (5d2, S=1) moments fluctuate dynamically, while their average effective moments undergo long-range order. In the second AFM phase below TN2=67 K, cobalt moments first become frozen and induce a noncollinear spin-canted AFM state, while dynamically fluctuating osmium moments are later frozen into a randomly canted state at…
Linear and nonlinear spin dynamics in multi-domain magnetoelastic antiferromagnets
2021
Antiferromagnets have recently surged as the prominent material platform for the next generation spintronics devices. Despite the remarkable abundance of antiferromagnets and the variety of their spin textures in nature, they share a widely common, if not ubiquitous, feature. Magnetoelasticity, which is expressed as strictions of different origin, relativistic and/or exchange, significantly contributes to the magnetic anisotropy of antiferromagnets. Crucially, a general theoretical framework able to address the role of domain walls on the spin dynamics in antiferromagnets in the presence of magnetoelasticity is lacking. Here we tackle this problem developing a very general macroscopic pheno…
Accessing the fundamentals of magnetotransport in metals with terahertz probes
2015
Spin-dependent conduction in metals underlies all modern magnetic memory technologies, such as giant magnetoresistance (GMR). The charge current in ferromagnetic transition metals is carried by two non-mixing populations of sp-band Fermi-level electrons: one of majority-spin and one of minority-spin. These electrons experience spin-dependent momentum scattering with localized electrons, which originate from the spin-split d-band. The direct observation of magnetotransport under such fundamental conditions, however, requires magnetotransport measurements on the same timescale as the electron momentum scattering, which takes place in the sub-100 fs regime. Using terahertz electromagnetic prob…
Chapter 23. Singlet Order in Heteronuclear Spin Systems
2020
The concept of heteronuclear Long-Lived spin States (LLSs) is introduced. In the simplest case of a pair of heteronuclei, such states are given by the singlet order of the spin pair, which can be efficiently sustained under Zero or Ultra-Low Field (ZULF) conditions. Here we describe two possible ways of detecting long-lived singlet order of heteronuclei: detection at ZULF conditions and NMR (Nuclear Magnetic Resonance) detection at high field utilising fast field-cycling. A theoretical description of the underlying spin dynamics is presented for both cases; the discussion is supported by experimental examples of LLSs in 13CH groups. The generality of these phenomena is discussed, as well as…
Dzyaloshinskii-Moriya and dipole-dipole interactions affect coupling-based Landau-Majorana-Stückelberg-Zener transitions
2020
It has been theoretically demonstrated that two spins (qubits or qutrits), coupled by exchange interaction only, undergo a coupling-based joint Landau-Majorana-St\"uckelberg-Zener (LMSZ) transition when a linear ramp acts upon one of the two spins. Such a transition, under appropriate conditions on the parameters, drives the two-spin system toward a maximally entangled state. In this paper, effects on the quantum dynamics of the two qudits, stemming from the Dzyaloshinskii-Moriya (DM) and dipole-dipole (d-d) interactions, are investigated qualitatively and quantitatively. The enriched Hamiltonian model of the two spins, shares with the previous microscopic one the same C2-symmetry which onc…
Tuning non-Markovianity by spin-dynamics control
2013
We study the interplay between forgetful and memory-keeping evolution enforced on a two-level system by a multi-spin environment whose elements are coupled to local bosonic baths. Contrarily to the expectation that any non-Markovian effect would be buried by the forgetful mechanism induced by the spin-bath coupling, one can actually induce a full Markovian-to-non-Markovian transition of the two-level system's dynamics, controllable by parameters such as the mismatch between the energy of the two-level system and of the spin environment. For a symmetric coupling, the amount of non-Markovianity surprisingly grows with the number of decoherence channels.
Towards peptide-based tunable multistate memristive materials
2021
Development of new memristive hardware is a technological requirement towards widespread neuromorphic computing. Molecular spintronics seems to be a fertile field for the design and preparation of this hardware. Within molecular spintronics, recent results on metallopeptides demonstrating the interaction between paramagnetic ions and the chirality induced spin selectivity effect hold particular promise for developing fast (ns–μs) operation times. [R. Torres-Cavanillas et al., J. Am. Chem. Soc., 2020, DOI: 10.1021/jacs.0c07531]. Among the challenges in the field, a major highlight is the difficulty in modelling the spin dynamics in these complex systems, but at the same time the use of inexp…